One-step fabrication of β-cyclodextrin modified magnetic graphene oxide nanohybrids for adsorption of Pb(II), Cu(II) and methylene blue in aqueous solutions | |
Ma, Ying-Xia1; Shao, Wen-Jie1; Sun, Wen1; Kou, Ya-Lan1; Li, Xin1; Yang, Hai-Peng2 | |
刊名 | Applied Surface Science |
2018-11-30 | |
卷号 | 459页码:544-553 |
关键词 | Adsorption Aromatic compounds Chlorination Chlorine compounds Cyclodextrins Fabrication Fourier transform infrared spectroscopy Graphene Heavy metals Iron compounds Lead compounds Magnetism Metal ions Nanostructured materials Precipitation (chemical) Scanning electron microscopy Sodium hydroxide Sulfur compounds Thermogravimetric analysis Transmission electron microscopy X ray photoelectron spectroscopy Adsorption capacities Adsorption properties Coprecipitation method Ferric chloride hexahydrate Methylene Blue Pseudo-second order model Vibrating sample magnetometer Zeta potential analysis |
ISSN号 | 01694332 |
DOI | 10.1016/j.apsusc.2018.08.025 |
英文摘要 | In this study, using graphene oxide (GO) as carrier, ferrous sulfate heptahydrate (FeSO4·7H2O) and ferric chloride hexahydrate (FeCl3·6H2O) as iron sources, sodium hydroxide (NaOH) as precipitant, β-cyclodextrin (β-CD) as a modifier, β-cyclodextrin modified magnetic graphene oxide (β-CD/MGO) nanohybrids were fabricated by a simple one-step reverse phase co-precipitation method. The as-prepared β-CD/MGO nanohybrids were characterized by transmission electron microscope (TEM), scanning electron microscope (SEM), X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), thermogravimetric analysis (TGA), vibrating sample magnetometer (VSM), N2 adsorption/desorption isotherm, X-ray photoelectron spectroscopy (XPS) and Zeta potential analysis. Simultaneously, the adsorption properties of the β-CD/MGO nanohybrids for Pb(II), Cu(II) heavy metal ions and methylene blue (MB) in single aqueous solution were explored by batch experiments. The results revealed that the β-CD/MGO nanohybrids with high superparamagnetism were successfully fabricated, the maximum adsorption capacities of β-CD/MGO nanohybrids for Pb(II), Cu(II) and MB were 279.21, 51.29 and 93.97 mg·g−1 at 298 K, respectively. The adsorption process could be better fitted by pseudo-second-order model and Langmuir model. © 2018 Elsevier B.V. |
资助项目 | State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals[18LHPY005] |
WOS研究方向 | Chemistry ; Materials Science ; Physics |
语种 | 英语 |
出版者 | Elsevier B.V., Netherlands |
WOS记录号 | WOS:000444600300069 |
状态 | 已发表 |
内容类型 | 期刊论文 |
源URL | [http://ir.lut.edu.cn/handle/2XXMBERH/114738] |
专题 | 省部共建有色金属先进加工与再利用国家重点实验室 材料科学与工程学院 |
通讯作者 | Ma, Ying-Xia |
作者单位 | 1.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Sch Mat Sci & Engn, Lanzhou 730050, Gansu, Peoples R China 2.Shenzhen Univ, Coll Mat Sci & Engn, Guangdong Res Ctr Interfacial Engn Funct Mat, Shenzhen 518060, Peoples R China |
推荐引用方式 GB/T 7714 | Ma, Ying-Xia,Shao, Wen-Jie,Sun, Wen,et al. One-step fabrication of β-cyclodextrin modified magnetic graphene oxide nanohybrids for adsorption of Pb(II), Cu(II) and methylene blue in aqueous solutions[J]. Applied Surface Science,2018,459:544-553. |
APA | Ma, Ying-Xia,Shao, Wen-Jie,Sun, Wen,Kou, Ya-Lan,Li, Xin,&Yang, Hai-Peng.(2018).One-step fabrication of β-cyclodextrin modified magnetic graphene oxide nanohybrids for adsorption of Pb(II), Cu(II) and methylene blue in aqueous solutions.Applied Surface Science,459,544-553. |
MLA | Ma, Ying-Xia,et al."One-step fabrication of β-cyclodextrin modified magnetic graphene oxide nanohybrids for adsorption of Pb(II), Cu(II) and methylene blue in aqueous solutions".Applied Surface Science 459(2018):544-553. |
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