In-situ sulfurized In2S3_MoO3@MoS2 heterojunction for visible light induced CO2 photoreduction | |
Wang, Fuhai; Liu, Daixin; Wen, Jing; Zheng, Xiaogang | |
刊名 | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING |
2021-10 | |
卷号 | 9期号:5 |
DOI | 10.1016/j.jece.2021.106042 |
英文摘要 | In2S3-decorated MoO3@MoS2 (In/MoO3@MoS2) composites were fabricated via the in-situ sulfurization of nonthermal plasma for the visible light driven photoreduction of CO2 to CH4 and CO. In2S3 can efficiently enhance the photocatalytic activity of In/MoO3@MoS2 in comparison to h-MoO3. The optimal 3-In/MoO3@MoS2 with a In content of 1.33% and the MoS2 thickness of around 10 nm presents the superior conversion efficiency of CO2, of which the yield of CH4 and CO are 29.4 and 35.6 mu mol g(-1) h (-1), respectively. However, the long-term photo-corrosion induced to the declining yield of CH4 and CO after three cycle times. The introduction of In2S3 into MoO3@MoS2 as well as the nonthermal plasma induced S-rich sites and O vacancies is likely to provide the sufficient active sites for promoting CO2 activation and the efficient junction interface for achieving the transfer and separation of charge carriers. |
内容类型 | 期刊论文 |
源URL | [http://ir.isl.ac.cn/handle/363002/34372] |
专题 | 青海盐湖研究所_盐湖资源与化学实验室 |
推荐引用方式 GB/T 7714 | Wang, Fuhai,Liu, Daixin,Wen, Jing,et al. In-situ sulfurized In2S3_MoO3@MoS2 heterojunction for visible light induced CO2 photoreduction[J]. JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING,2021,9(5). |
APA | Wang, Fuhai,Liu, Daixin,Wen, Jing,&Zheng, Xiaogang.(2021).In-situ sulfurized In2S3_MoO3@MoS2 heterojunction for visible light induced CO2 photoreduction.JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING,9(5). |
MLA | Wang, Fuhai,et al."In-situ sulfurized In2S3_MoO3@MoS2 heterojunction for visible light induced CO2 photoreduction".JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING 9.5(2021). |
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