Development of a 443 nm diode laser-based differential photoacoustic spectrometer for simultaneous measurements of aerosol absorption and NO2 | |
Cao, Yuan1,2; Liu, Qiang2; Wang, Ruifeng2; Liu, Kun2; Chen, Weidong3; Wang, Guishi2; Gao, Xiaoming1,2 | |
刊名 | PHOTOACOUSTICS |
2021-03-01 | |
卷号 | 21 |
关键词 | Photoacoustic spectrometer Absorption coefficient Aerosol Nitrogen dioxide |
ISSN号 | 2213-5979 |
DOI | 10.1016/j.pacs.2020.100229 |
通讯作者 | Liu, Kun(liukun@aiofm.ac.cn) ; Gao, Xiaoming(xmgao@aiofm.ac.cn) |
英文摘要 | Measurement of ambient aerosol and nitrogen dioxide (NO2) is important as they are major pollutants from the burning of fossil fuel and biomass. In the present work, a differential photoacoustic spectrometer (D-PAS) was developed for simultaneous, online measurements of aerosol optical absorption and NO2 concentration. A novel photoacoustic resonator was designed and employed in the D-PAS for controlling a large flow rate, improving response time, and keeping the flow noise at a low level. The detection limits of 1.0 Mm-1 and 0.87 ppb for aerosol absorption and NO2 concentration measurements were achieved with a lock-in amplifier time constant of 1 s. The D-PAS accuracy was demonstrated by performing a long-time, continuous measurement of aerosol, and NO2 in ambient air. The measured results of NO2 are consistent with the NOx analyzer and environmental monitoring station results. |
资助项目 | National Natural Science Foundation of China[41475023] ; National Natural Science Foundation of China[41730103] ; National Natural Science Foundation of China[41575030] ; National Key Research and Development Program of China[2016YFC0303900] ; National Key Research and Development Program of China[2017YFC0209700] |
WOS关键词 | OPTICAL-PROPERTIES ; LIGHT-ABSORPTION ; NITROGEN-DIOXIDE ; SPECTROSCOPY ; CALIBRATION ; UV ; SOOT ; CELL |
WOS研究方向 | Acoustics ; Engineering ; Instruments & Instrumentation ; Radiology, Nuclear Medicine & Medical Imaging |
语种 | 英语 |
出版者 | ELSEVIER GMBH |
WOS记录号 | WOS:000653150000003 |
资助机构 | National Natural Science Foundation of China ; National Key Research and Development Program of China |
内容类型 | 期刊论文 |
源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/122668] |
专题 | 中国科学院合肥物质科学研究院 |
通讯作者 | Liu, Kun; Gao, Xiaoming |
作者单位 | 1.Univ Sci & Technol China, Sch Environm Sci & Optoelect Technol, Hefei 230031, Peoples R China 2.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, HFIPS, Hefei 230031, Peoples R China 3.Univ Littoral Cote dOpale, Lab Physicochim Atmosphere, 189A Av Maurice Schumann, F-59140 Dunkerque, France |
推荐引用方式 GB/T 7714 | Cao, Yuan,Liu, Qiang,Wang, Ruifeng,et al. Development of a 443 nm diode laser-based differential photoacoustic spectrometer for simultaneous measurements of aerosol absorption and NO2[J]. PHOTOACOUSTICS,2021,21. |
APA | Cao, Yuan.,Liu, Qiang.,Wang, Ruifeng.,Liu, Kun.,Chen, Weidong.,...&Gao, Xiaoming.(2021).Development of a 443 nm diode laser-based differential photoacoustic spectrometer for simultaneous measurements of aerosol absorption and NO2.PHOTOACOUSTICS,21. |
MLA | Cao, Yuan,et al."Development of a 443 nm diode laser-based differential photoacoustic spectrometer for simultaneous measurements of aerosol absorption and NO2".PHOTOACOUSTICS 21(2021). |
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