Development of a 443 nm diode laser-based differential photoacoustic spectrometer for simultaneous measurements of aerosol absorption and NO2
Cao, Yuan1,2; Liu, Qiang2; Wang, Ruifeng2; Liu, Kun2; Chen, Weidong3; Wang, Guishi2; Gao, Xiaoming1,2
刊名PHOTOACOUSTICS
2021-03-01
卷号21
关键词Photoacoustic spectrometer Absorption coefficient Aerosol Nitrogen dioxide
ISSN号2213-5979
DOI10.1016/j.pacs.2020.100229
通讯作者Liu, Kun(liukun@aiofm.ac.cn) ; Gao, Xiaoming(xmgao@aiofm.ac.cn)
英文摘要Measurement of ambient aerosol and nitrogen dioxide (NO2) is important as they are major pollutants from the burning of fossil fuel and biomass. In the present work, a differential photoacoustic spectrometer (D-PAS) was developed for simultaneous, online measurements of aerosol optical absorption and NO2 concentration. A novel photoacoustic resonator was designed and employed in the D-PAS for controlling a large flow rate, improving response time, and keeping the flow noise at a low level. The detection limits of 1.0 Mm-1 and 0.87 ppb for aerosol absorption and NO2 concentration measurements were achieved with a lock-in amplifier time constant of 1 s. The D-PAS accuracy was demonstrated by performing a long-time, continuous measurement of aerosol, and NO2 in ambient air. The measured results of NO2 are consistent with the NOx analyzer and environmental monitoring station results.
资助项目National Natural Science Foundation of China[41475023] ; National Natural Science Foundation of China[41730103] ; National Natural Science Foundation of China[41575030] ; National Key Research and Development Program of China[2016YFC0303900] ; National Key Research and Development Program of China[2017YFC0209700]
WOS关键词OPTICAL-PROPERTIES ; LIGHT-ABSORPTION ; NITROGEN-DIOXIDE ; SPECTROSCOPY ; CALIBRATION ; UV ; SOOT ; CELL
WOS研究方向Acoustics ; Engineering ; Instruments & Instrumentation ; Radiology, Nuclear Medicine & Medical Imaging
语种英语
出版者ELSEVIER GMBH
WOS记录号WOS:000653150000003
资助机构National Natural Science Foundation of China ; National Key Research and Development Program of China
内容类型期刊论文
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/122668]  
专题中国科学院合肥物质科学研究院
通讯作者Liu, Kun; Gao, Xiaoming
作者单位1.Univ Sci & Technol China, Sch Environm Sci & Optoelect Technol, Hefei 230031, Peoples R China
2.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, HFIPS, Hefei 230031, Peoples R China
3.Univ Littoral Cote dOpale, Lab Physicochim Atmosphere, 189A Av Maurice Schumann, F-59140 Dunkerque, France
推荐引用方式
GB/T 7714
Cao, Yuan,Liu, Qiang,Wang, Ruifeng,et al. Development of a 443 nm diode laser-based differential photoacoustic spectrometer for simultaneous measurements of aerosol absorption and NO2[J]. PHOTOACOUSTICS,2021,21.
APA Cao, Yuan.,Liu, Qiang.,Wang, Ruifeng.,Liu, Kun.,Chen, Weidong.,...&Gao, Xiaoming.(2021).Development of a 443 nm diode laser-based differential photoacoustic spectrometer for simultaneous measurements of aerosol absorption and NO2.PHOTOACOUSTICS,21.
MLA Cao, Yuan,et al."Development of a 443 nm diode laser-based differential photoacoustic spectrometer for simultaneous measurements of aerosol absorption and NO2".PHOTOACOUSTICS 21(2021).
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