Sewage sludge in microwave oven: A sustainable synthetic approach toward carbon dots for fluorescent sensing of para-Nitrophenol
Hu, Yaoping; Gao, Zhijin
刊名JOURNAL OF HAZARDOUS MATERIALS
2020
卷号382
关键词GRAPHENE QUANTUM DOTS CHAIN FATTY-ACIDS GREEN SYNTHESIS HYDROTHERMAL TREATMENT FORMATION MECHANISM P-NITROPHENOL WASTE PAPER NITROGEN SULFUR 4-NITROPHENOL
DOI10.1016/j.jhazmat.2019.121048
英文摘要Million tons of sewage sludge produced yearly creates a severe pollution problem to environment, and thus needs either to be properly disposed of, or recovered. Here, we demonstrate a value-added utilization of sewage sludge by converting its contained organics into nanosized carbon dots (CDs) with microwave irradiation. This synthetic method, using waste resources as precursors and avoiding the requirement of hazardous reagents and complex procedures, has the great advantage of low cost, environmental friendliness, and easy scalability. The resultant CDs exhibit excellent fluorescence properties with a large quantum yield (QY) of up to 21.7%, higher than the most values of waste-derived CDs. It is found that CDs can serve as a sensitive and selective sensor to detect para-Nitrophenol (p-NP), a toxic pollutant, through fluorescence quenching, giving a linear detection range of 0.2-20 mu M and a detection limit of as low as 0.069 mu M. Systematic investigations suggest that the inner filter effect (IFE) is the dominant sensing mechanism. Moreover, the practical applications of CDs for p-NP assay in real water samples achieve good results.
学科主题Engineering ; Environmental Sciences & Ecology
内容类型期刊论文
源URL[http://ir.nimte.ac.cn/handle/174433/20189]  
专题2020专题
作者单位Hu, YP (corresponding author), Ningbo Univ, Sch Mat Sci & Chem Engn, Ningbo 315211, Zhejiang, Peoples R China.
推荐引用方式
GB/T 7714
Hu, Yaoping,Gao, Zhijin. Sewage sludge in microwave oven: A sustainable synthetic approach toward carbon dots for fluorescent sensing of para-Nitrophenol[J]. JOURNAL OF HAZARDOUS MATERIALS,2020,382.
APA Hu, Yaoping,&Gao, Zhijin.(2020).Sewage sludge in microwave oven: A sustainable synthetic approach toward carbon dots for fluorescent sensing of para-Nitrophenol.JOURNAL OF HAZARDOUS MATERIALS,382.
MLA Hu, Yaoping,et al."Sewage sludge in microwave oven: A sustainable synthetic approach toward carbon dots for fluorescent sensing of para-Nitrophenol".JOURNAL OF HAZARDOUS MATERIALS 382(2020).
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