Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers

doi:10.1016/j.scitotenv.2020.141829

CORC > 烟台海岸带研究所 > 中国科学院烟台海岸带研究所 > 山东省海岸带环境工程技术研究中心

	Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers
	Jiang, Ming 1,2; Sheng, Yanqing 2; Liu, Qunqun 1,2; Wang, Wenjing 2; Liu, Xiaozhu 1,2
刊名	SCIENCE OF THE TOTAL ENVIRONMENT
	2021-01-15
卷号	752 页码:11
关键词	Coastal rivers Sediment Inorganic sulfur Organic sulfur Buffer capacity
ISSN号	0048-9697
DOI	10.1016/j.scitotenv.2020.141829
通讯作者	Sheng, Yanqing(yqsheng@yic.ac.cn)
英文摘要	Geochemical processes of sulfur (S) in river aquatic systems play a crucial role in environmental evolution. In this study, the distributions and sources of reduced inorganic sulfur (RIS) and organic sulfur (OS) in coastal river surface sediments were investigated. The results indicated that OS dominated total S (80%), and OS (i.e., humic acid sulfur, HAS; fulvic acid sulfur, FAS) correlated with the availability of labile organic matter (OM) and reactive iron (Fe). Terrigenous inputs and sulfurization contributed to the enrichment of FAS through the S reduction. Autochthonous biological inputs were potential sources of HAS from S oxidization. The X-ray photoelectron spectroscopy showed that the main sources of S in surface sediments were deposited as the form of organic ester-sulfate. Aquatic life could break S down further, producing reduced S compounds accumulated as thiols and RIS in anoxic sediments. RIS was dominated by acid volatile sulfur (AVS) and chromium (II)-reducible sulfur (CRS). Reactive Fe oxides were major control factors for the conversation from hydrogen sulfide (H2S) to AVS, whereas elemental sulfide (ES) controlled the conversion from AVS into CRS in coastal rivers. (C) 2020 Elsevier B.V. All rights reserved.
资助项目	Strategic Priority Research Program of the Chinese Academy of Sciences[XDA23050203] ; National Natural Science Foundation of China[41373100] ; Key Project of Research and Development Plan of Yantai[2018ZHGY080] ; Key Research and Development Program of Shandong Province[2019GSF109002]
WOS关键词	BUFFERING CAPACITY ; SPATIAL-DISTRIBUTION ; REACTIVE IRON ; JIAOZHOU BAY ; HUMIC SULFUR ; PHOSPHORUS ; DIAGENESIS ; SULFIDE ; ACCUMULATION ; ENRICHMENT
WOS研究方向	Environmental Sciences & Ecology
语种	英语
WOS记录号	WOS:000588243900049
资助机构	Strategic Priority Research Program of the Chinese Academy of Sciences ; National Natural Science Foundation of China ; Key Project of Research and Development Plan of Yantai ; Key Research and Development Program of Shandong Province
内容类型	期刊论文
源URL	[http://ir.yic.ac.cn/handle/133337/28287]
专题	烟台海岸带研究所_山东省海岸带环境工程技术研究中心烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
通讯作者	Sheng, Yanqing
作者单位	1.Univ Chinese Acad Sci, Beijing, Peoples R China 2.Chinese Acad Sci, Res Ctr Coastal Environm Engn Technol Shandong Pr, Yantai Inst Coastal Zone Res, Yantai, Peoples R China
推荐引用方式 GB/T 7714	Jiang, Ming,Sheng, Yanqing,Liu, Qunqun,et al. Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2021,752:11.
APA	Jiang, Ming,Sheng, Yanqing,Liu, Qunqun,Wang, Wenjing,&Liu, Xiaozhu.(2021).Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers.SCIENCE OF THE TOTAL ENVIRONMENT,752,11.
MLA	Jiang, Ming,et al."Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers".SCIENCE OF THE TOTAL ENVIRONMENT 752(2021):11.